In general, yes. Remember there are 6 total shim stacks under the bonnet to account for. If you increase the shims, the upper front door gap will decrease...but less than the lower front door gap, which may not change at all. The bumper supports also have to be loosened, as the bumpers bolt to both the frame and the body.
The relation is not direct. That is, the process is that when you increase the shims, the fwd scuttle leans back, which reduces the clearance at the lower rear bottom edge of the door and the upper rear of the door. The hinge keeps the front of the door where it started. Then, if you adjust the door hinges, you can average out the gaps and level the bottom of the door.
If it sounds like a can of worms, it can be if you don't think through what will happen ahead of time...
John